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2013
2023
2023
2017
Siberian Arctic black carbon: gas flaring and wildfire impact
As explained in the latest Arctic Monitoring and Assessment Programme (AMAP) report released in early 2021, the Arctic has warmed 3 times more quickly than the planet as a whole, as well as faster than previously thought. The Siberian Arctic is of great interest mainly because observations are sparse or largely lacking. A research aerosol station has been developed on Bely Island (Kara Sea) in western Siberia. Measurements of equivalent black carbon (EBC) concentrations were carried out at the “Island Bely” station continuously from August 2019 to November 2020. The source origin of the measured EBC and the main contributing sources were assessed using atmospheric transport modeling coupled with the most updated emission inventories for anthropogenic and biomass burning sources of BC.
The obtained climatology for BC during the period of measurements showed an apparent seasonal variation with the highest concentrations between December and April (60 ± 92 ng m−3) and the lowest between June and September (18 ± 72 ng m−3), typical of the Arctic haze seasonality reported elsewhere. When air masses arrived at the station through the biggest oil and gas extraction regions of Kazakhstan, Volga-Ural, Komi, Nenets and western Siberia, BC contribution from gas flaring dominated over domestic, industrial and traffic sectors, ranging from 47 % to 68 %, with a maximum contribution in January. When air was transported from Europe during the cold season, emissions from transportation were more important. Accordingly, shipping emissions increased due to the touristic cruise activities and the ice retreat in summertime. Biomass burning (BB) played the biggest role between April and October, contributing 81 % at maximum in July. Long-range transport of BB aerosols appeared to induce large variability to the absorption Ångström exponent (AAE) with values > 1.0 (excluding outliers). As regards the continental contribution to surface BC at the Island Bely station, Russian emissions dominated during the whole year, while European and Asian ones contributed up to 20 % in the cold period. Quantification of several pollution episodes showed an increasing trend in surface concentrations and frequency during the cold period as the station is directly in the Siberian gateway of the highest anthropogenic pollution sources to the Russian Arctic.
2022
2009
Signals from the south; humpback whales carry messages of Antarctic sea‐ice ecosystem variability
John Wiley & Sons
2018
Signatures of climate tele-connection patterns in geophysical data series from Northern Scandinavia. NILU F
2003
Polluted air is a major global health risk factor, yet the chemical composition and toxicity of airborne gases and particles remain underexplored due to their complexity and difficulties in sampling. We recently introduced how polydimethylsiloxane (PDMS) foam─or silicone foam─can be synthesized for passive air sampling, enabling simple and cost-effective nontarget chemical profiling of indoor air. Here, we demonstrate expanded applications, indoors and outdoors, with commercial PDMS-foam, including for: (i) wide-scope target analysis of >220 priority substances by quantitative liquid- and gas chromatography-high-resolution mass spectrometry, (ii) microscopic characterization and nontarget profiling of accumulated fine particles, and (iii) effect-guided discovery of harmful substances, combining toxicological data with nontarget analysis in silico. Median method quantification limits were 0.12 ng/mL, 90% of target analytes had absolute recoveries between 70 and 130%, and hazardous substances were discovered, including ethylene glycols, insecticides, and UV filters. Microscopy revealed the accumulation of abundant fine particles, and the automated characterization of the fluorescent fraction revealed that most were <4 μm. Extracts from outdoor samples reduced human lung cell viability, and multivariate modeling flagged families of potentially toxic substances in a virtual effect-directed analysis. PDMS-foam disks require field calibration to determine their linear sampling rate(s), but current results and applications establish PDMS-foam as a multimodal passive sampler, enabling integrated chemical quantitation, toxicological analysis, and molecular discovery in air.
2026
2012
Simplified models for integrated air quality management in urban areas. NATO science for peace and security series
2008
Interdecadal change in the relationship between the East Asian winter monsoon (EAWM) and the Arctic Oscillation (AO) has been documented by many studies. This study, utilizing the model outputs from phase 5 of the Coupled Model Intercomparison Project (CMIP5), evaluates the ability of the coupled models in CMIP5 to capture the intensified relationship between the EAWM and winter AO since the 1980s, and further projects the evolution of the EAWM–AO relationship during the 21st century. It is found that the observed evolution of the EAWM–AO relationship can be reproduced well by some coupled models (e.g., GFDL-ESM2M, GISS-E2-H, and MPI-ESM-MR). The coupled models’ simulations indicate that the impact of winter AO on the EAWM-related circulation and East Asian winter temperature has strengthened since the 1980s. Such interdecadal change in the EAWM–AO relationship is attributed to the intensified propagation of stationary planetary waves associated with winter AO. Projections under the RCP4.5 and RCP8.5 scenarios suggest that the EAWM–AO relationship is significant before the 2030s and after the early 2070s, and insignificant during the 2060s, but uncertain from the 2030s to the 2050s.
2018
2005